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Trayvon Isiah Willingham was booked for murder Monday, according to the department. His bail has been set at $2 million.
Police believe Willingham and 62-year-old Darryl Winborn were arguing on the bus last Thursday when Willingham pepper-sprayed the other man and took off.
Man dies after being pepper sprayed during altercation on Metro bus in Koreatown
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Winborn wound up dying at the scene, but an official cause of death has not been released.
Details about what led up to the deadly altercation were not available.